Synthetic studies of centromere-associated protein-E (CENP-E) inhibitors: 1.Exploration of fused bicyclic core scaffolds using electrostatic potential map

Bioorg Med Chem. 2013 Sep 1;21(17):5488-502. doi: 10.1016/j.bmc.2013.05.067. Epub 2013 Jun 11.

Abstract

Centromere-associated protein-E (CENP-E), a mitotic kinesin that plays an important role in mitotic progression, is an attractive target for cancer therapeutic drugs. For the purpose of developing novel CENP-E inhibitors as cancer therapeutics, we investigated a fused bicyclic compound identified by high throughput screening, 4-oxo-4,5-dihydrothieno[3,4-c]pyridine-6-carboxamide 1a. Based on this scaffold, we designed inhibitors for efficient binding at the L5 site in CENP-E utilizing homology modeling as well as electrostatic potential map (EPM) analysis to enhance CENP-E inhibitory activity. This resulted in a new lead, 5-bromoimidazo[1,2-a]pyridine 7, which showed potent CENP-E enzyme inhibition (IC50: 50nM) and cellular activity with accumulation of phosphorylated histone H3 in HeLa cells. Our homology model and EPM analysis proved to be useful tools for the rational design of CENP-E inhibitors.

Keywords: (1)H NMR; 4-Oxo-4,5-dihydrothieno[3,4-c]pyridine-6-carboxamide; CENP-E; DSC; EPM; Electrostatic potential map (EPM); Imidazo[1,2-a]pyridine; PD; SAR; ZATPRXWLTXOXAQ-UHFFFAOYSA-N; centromere-associated protein-E; differential scanning calorimetry; electrostatic potential map; pharmacodynamic; proton nuclear magnetic resonance; structure–activity relationship.

MeSH terms

  • Amides / chemical synthesis*
  • Amides / chemistry
  • Amides / metabolism
  • Binding Sites
  • Bridged Bicyclo Compounds / chemistry*
  • Chromosomal Proteins, Non-Histone / antagonists & inhibitors*
  • Chromosomal Proteins, Non-Histone / metabolism
  • HeLa Cells
  • Histones / metabolism
  • Humans
  • Imidazoles / chemical synthesis*
  • Imidazoles / chemistry
  • Imidazoles / metabolism
  • Molecular Docking Simulation
  • Protein Binding
  • Protein Structure, Tertiary
  • Pyridines / chemical synthesis*
  • Pyridines / chemistry
  • Pyridines / metabolism
  • Static Electricity
  • Structure-Activity Relationship

Substances

  • 5-bromoimidazo(1,2-a)pyridine
  • Amides
  • Bridged Bicyclo Compounds
  • Chromosomal Proteins, Non-Histone
  • Histones
  • Imidazoles
  • Pyridines
  • centromere protein E